General Synthesis of Single-Atom Catalysts for Hydrogen Evolution Reactions and Room-Temperature Na-S Batteries.

Lai, W-H; Wang, H; Zheng, L; Jiang, Q; Yan, Z-C; Wang, L; Yoshikawa, H; Matsumura, D; Sun, Q; Wang, Y-X; Gu, Q; Wang, J-Z; Liu, H-K; Chou, S-L; Dou, S-X

General Synthesis of Single-Atom Catalysts for Hydrogen Evolution Reactions and Room-Temperature Na-S Batteries.

Lai, W-H Wang, H Zheng, L Jiang, Q Yan, Z-C Wang, L Yoshikawa, H Matsumura, D Sun, Q Wang, Y-X Gu, Q Wang, J-Z Liu, H-K Chou, S-L Dou, S-X

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Publisher:: WILEY-V C H VERLAG GMBH
Publication Type:: Journal Article
Citation:: Angewandte Chemie (International ed. in English), 2020, 59, (49), pp. 22171-22178
Issue Date:: 2020-12

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Field	Value	Language
dc.contributor.author	Lai, W-H
dc.contributor.author	Wang, H
dc.contributor.author	Zheng, L
dc.contributor.author	Jiang, Q
dc.contributor.author	Yan, Z-C
dc.contributor.author	Wang, L
dc.contributor.author	Yoshikawa, H
dc.contributor.author	Matsumura, D
dc.contributor.author	Sun, Q
dc.contributor.author	Wang, Y-X
dc.contributor.author	Gu, Q
dc.contributor.author	Wang, J-Z
dc.contributor.author	Liu, H-K
dc.contributor.author	Chou, S-L
dc.contributor.author	Dou, S-X
dc.date.accessioned	2021-03-02T21:15:04Z
dc.date.available	2021-03-02T21:15:04Z
dc.date.issued	2020-12
dc.identifier.citation	Angewandte Chemie (International ed. in English), 2020, 59, (49), pp. 22171-22178
dc.identifier.issn	1433-7851
dc.identifier.issn	1521-3773
dc.identifier.uri	http://hdl.handle.net/10453/146651
dc.description.abstract	Herein, we report a comprehensive strategy to synthesize a full range of single-atom metals on carbon matrix, including V, Mn, Fe, Co, Ni, Cu, Ge, Mo, Ru, Rh, Pd, Ag, In, Sn, W, Ir, Pt, Pb, and Bi. The extensive applications of various SACs are manifested via their ability to electro-catalyze typical hydrogen evolution reactions (HER) and conversion reactions in novel room-temperature sodium sulfur batteries (RT-Na-S). The enhanced performances for these electrochemical reactions arisen from the ability of different single active atoms on local structures to tune their electronic configuration. Significantly, the electrocatalytic behaviors of diverse SACs, assisted by density functional theory calculations, are systematically revealed by in situ synchrotron X-ray diffraction and in situ transmission electronic microscopy, providing a strategic library for the general synthesis and extensive applications of SACs in energy conversion and storage.
dc.format	Print-Electronic
dc.language	eng
dc.publisher	WILEY-V C H VERLAG GMBH
dc.relation.ispartof	Angewandte Chemie (International ed. in English)
dc.relation.isbasedon	10.1002/anie.202009400
dc.rights	info:eu-repo/semantics/closedAccess
dc.subject	03 Chemical Sciences
dc.subject.classification	Organic Chemistry
dc.title	General Synthesis of Single-Atom Catalysts for Hydrogen Evolution Reactions and Room-Temperature Na-S Batteries.
dc.type	Journal Article
utslib.citation.volume	59
utslib.location.activity	Germany
utslib.for	03 Chemical Sciences
pubs.organisational-group	/University of Technology Sydney/Faculty of Science
pubs.organisational-group	/University of Technology Sydney/Faculty of Science/School of Mathematical and Physical Sciences
pubs.organisational-group	/University of Technology Sydney
utslib.copyright.status	closed_access	*
dc.date.updated	2021-03-02T21:15:02Z
pubs.issue	49
pubs.publication-status	Published
pubs.volume	59
utslib.citation.issue	49

Abstract:

Herein, we report a comprehensive strategy to synthesize a full range of single-atom metals on carbon matrix, including V, Mn, Fe, Co, Ni, Cu, Ge, Mo, Ru, Rh, Pd, Ag, In, Sn, W, Ir, Pt, Pb, and Bi. The extensive applications of various SACs are manifested via their ability to electro-catalyze typical hydrogen evolution reactions (HER) and conversion reactions in novel room-temperature sodium sulfur batteries (RT-Na-S). The enhanced performances for these electrochemical reactions arisen from the ability of different single active atoms on local structures to tune their electronic configuration. Significantly, the electrocatalytic behaviors of diverse SACs, assisted by density functional theory calculations, are systematically revealed by in situ synchrotron X-ray diffraction and in situ transmission electronic microscopy, providing a strategic library for the general synthesis and extensive applications of SACs in energy conversion and storage.

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http://hdl.handle.net/10453/146651