Field |
Value |
Language |
dc.contributor.author |
Lu, J |
|
dc.contributor.author |
Wang, T |
|
dc.contributor.author |
Yang, J |
|
dc.contributor.author |
Shen, X |
|
dc.contributor.author |
Pang, H |
|
dc.contributor.author |
Sun, B
https://orcid.org/0000-0002-4365-486X
|
|
dc.contributor.author |
Wang, G
https://orcid.org/0000-0003-4295-8578
|
|
dc.contributor.author |
Wang, C |
|
dc.date.accessioned |
2025-03-20T03:20:43Z |
|
dc.date.available |
2025-03-20T03:20:43Z |
|
dc.date.issued |
2024-10-14 |
|
dc.identifier.citation |
Angewandte Chemie, 2024, 136, (42) |
|
dc.identifier.issn |
0044-8249 |
|
dc.identifier.issn |
1521-3757 |
|
dc.identifier.uri |
http://hdl.handle.net/10453/186036
|
|
dc.description.abstract |
<jats:title>Abstract</jats:title><jats:p>Rechargeable aqueous zinc‐ion (Zn‐ion) batteries are widely regarded as important candidates for next‐generation energy storage systems for low‐cost renewable energy storage. However, the development of Zn‐ion batteries is currently facing significant challenges due to uncontrollable Zn dendrite growth and severe parasitic reactions on Zn metal anodes. Herein, we report an effective strategy to improve the performance of aqueous Zn‐ion batteries by leveraging the self‐assembly of bovine serum albumin (BSA) into a bilayer configuration on Zn metal anodes. BSA′s hydrophilic and hydrophobic fragments form unique and intelligent ion channels, which regulate the migration of Zn ions and facilitate their desolvation process, significantly diminishing parasitic reactions on Zn anodes and leading to a uniform Zn deposition along the Zn (002) plane. Notably, the Zn||Zn symmetric cell with BSA as the electrolyte additive demonstrated a stable cycling performance for up to 2400 hours at a high current density of 10 mA cm<jats:sup>−2</jats:sup>. This work demonstrates the pivotal role of self‐assembled protein bilayer structures in improving the durability of Zn anodes in aqueous Zn‐ion batteries.</jats:p> |
|
dc.language |
en |
|
dc.publisher |
Wiley |
|
dc.relation |
http://purl.org/au-research/grants/arc/DP230101579
|
|
dc.relation.ispartof |
Angewandte Chemie |
|
dc.relation.isbasedon |
10.1002/ange.202409838 |
|
dc.rights |
info:eu-repo/semantics/openAccess |
|
dc.subject |
03 Chemical Sciences |
|
dc.subject.classification |
Organic Chemistry |
|
dc.subject.classification |
34 Chemical sciences |
|
dc.title |
Multifunctional Self‐Assembled Bio‐Interfacial Layers for High‐Performance Zinc Metal Anodes |
|
dc.type |
Journal Article |
|
utslib.citation.volume |
136 |
|
utslib.for |
03 Chemical Sciences |
|
pubs.organisational-group |
University of Technology Sydney |
|
pubs.organisational-group |
University of Technology Sydney/Faculty of Science |
|
pubs.organisational-group |
University of Technology Sydney/Faculty of Science/School of Mathematical and Physical Sciences |
|
pubs.organisational-group |
University of Technology Sydney/UTS Groups |
|
pubs.organisational-group |
University of Technology Sydney/UTS Groups/Centre for Clean Energy Technology (CCET) |
|
utslib.copyright.status |
open_access |
* |
dc.rights.license |
This work is licensed under a Creative Commons Attribution 4.0 International License (CC BY 4.0). To view a copy of this license, visit https://creativecommons.org/licenses/by/4.0/ |
|
dc.date.updated |
2025-03-20T03:20:41Z |
|
pubs.issue |
42 |
|
pubs.publication-status |
Published |
|
pubs.volume |
136 |
|
utslib.citation.issue |
42 |
|